The dancehall legend heated up the NPR offices with a wide-ranging set of hits from his career.
The departure of Boilen, who also created and hosts All Songs Considered, follows news that two other high-level executives will soon exit the broadcaster.
"I'm Chloe -- Miss Bailey if you nasty."
The sibling trio are currently on their first-ever U.S. tour.
He reached back for mixtape song "seoul" and played a pair of tracks from his new "Indigo" solo album.